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Recently, dielectric metasurfaces, in addition to their use as lenses and for spatially shaping the phase and polarization of light on the nanoscale 12, 13, 14, 15, were employed in an angular-dispersive Fourier-transform setup 16, providing fine-grained control of the time-domain properties of ultrashort laser pulses. A key challenge in their application remains dispersion control: because all transparent materials are normally dispersive in the ultraviolet, visible, and near-infrared regions below a wavelength of 1.3 μm, the realization of compressed laser pulses currently requires complex angular-dispersive 5, 6, 7, reflective 8, 9, 10, or photonic-crystal-fiber-based compression setups 11, which all add significant complexity, path length, and beam deviations to the optical setup. Applying these coatings to conventional optics renders them ultrashort pulse compatible and suitable for a wide range of applications.įemtosecond light pulses are the basis for the highest achievable time resolutions and electrical field intensities today and have become central tools in microscopy 1, medicine 2, technology 3, and physical chemistry 4. We characterize the arrays’ performance in the spectral domain via white light interferometry and directly demonstrate the temporal compression of femtosecond laser pulses.
The coatings induce anomalous group delay dispersion in the visible to near-infrared spectral region around 800 nm wavelength over an 80 nm bandwidth. Here we experimentally demonstrate ultrathin nanostructured coatings that resolve this challenge: we tailor the dispersion of silicon nanopillar arrays such that they temporally reshape pulses upon transmission using slow light effects and act as ultrashort laser pulse compressors. One consequence is chromatic dispersion, i.e., light of different frequencies travels at different velocities, causing ultrashort laser pulses to elongate in time while propagating. Toutes les marques déposées, noms de produits et noms ou logos d'entreprises sont la propriété de leurs propriétaires respectifs.Transparent materials do not absorb light but have profound influence on the phase evolution of transmitted radiation.
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